Ultrafast Scanning Probe Microscopy
Ultrafast Scanning Probe Microscopy
Research Group Melanie Müller
Research Group Melanie Müller

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We are interested in the spatio-temporal response of solid state surfaces, nanostructures, and molecules following ultrafast laser excitation. Our goal is to obtain an atomistic understanding of photoinduced processes on (sub-) nanometer length and femtosecond time scales by employing novel pump-probe schemes for ultrafast scanning probe microscopy (SPM). We envision to study, drive and control solid state matter in highly non-equilibrium states on ultrashort length und ultrafast time scales.

To achieve this goal, we are putting efforts into the development of ultrafast scanning probe methods, with a strong focus on broadband THz-gated STM combined with femtosecond optical excitation and all-optical plasmon-assisted femtosecond STM. For more information please check our research page and follow our news below.

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New Paper: Femtosecond Thermal and Nonthermal Hot Electron Tunneling Inside a Photoexcited Tunnel Junction
Aug 2022
Is hot electron tunneling from a femtosecond laser-excited STM tip thermal or nonthermal? (How) do the femtosecond dynamics of hot electrons inside the tip affect the ultrafast photocurrent response in STM? We have addressed this fundamental question using a THz-gated STM and are pleased that our results are now being published in ACS Nano. (DOI: 10.1021/acsnano.2c04846)
STM meets coherent phonons: Watching coherent lattice vibrations in real-space
Jun 2022
Can photoexcited STM be used to probe ultrafast structural dynamics at surfaces? Yes, it can! Looking forward to present our new paper on “Nanoscale coherent phonon spectroscopy” soon. Thanks to Takashi Kumagai for the great collaboration! Coming out soon.
New preprint: Tracing hot electron tunneling in real-time
May 2022
We had a closer look into the nonequilibrium dynamics of hot electrons inside
a photoexcited STM tip, and were curious about the question: does the tunneling of photo-generated hot electrons in STM have thermal or nonthermal character? THz sampling inside the photoexcited STM junction can answer this question, have a closer look at our preprint: https://doi.org/10.48550/arXiv.2205.08248.
Alkisti joins as PhD student
May 2022
After her successful master, in which she optimized high-power operation of the spintronic THz emitter for THz-STM applications, Alkisti now joins us as a PhD student. She will work on phase-resolved THz studies inside STM junctions. Welcome (back) Alkisti!
New lab: Low-temperature THz-STM starts operation
May 2022
After dealing with various technical hurdles, we are finally back to STM operation in our new lab: with cryo and new laser system. Many thanks to the team for the great job to get this running! We are excited to see new data coming out of this machine soon!